Hydrogen Evolution Reactivity of Pentagonal Carbon Rings and p-d Orbital Hybridization Effect with Ru,Angewandte Chemie International Edition

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Hydrogen Evolution Reactivity of Pentagonal Carbon Rings and p-d Orbital Hybridization Effect with Ru
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-09-14 , DOI: 10.1002/anie.202411125
Lei Gong ₁ , Fanjie Xia ₁ , Jiawei Zhu ₁ , Xueqin Mu ₁ , Ding Chen ₁ , Hongyu Zhao ₁ , Lei Chen ₁ , Shichun Mu ₂

Affiliation

Topological pentagon defects endow carbon nanomaterial with intrinsic hydrogen evolution reactivity and draw forth a strong p-d orbital hybridization effect with Ru species, which induces favorable electron transfer and weakened hydrogen adsorption strength and reaction barrier of Ru sites, significantly driving electrocatalytic hydrogen production.

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