Black titanium oxide: synthesis, modification, characterization, physiochemical properties, and emerging applications for energy conversion and storage, and environmental sustainability,Chemical Society Reviews

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Black titanium oxide: synthesis, modification, characterization, physiochemical properties, and emerging applications for energy conversion and storage, and environmental sustainability
Chemical Society Reviews ( IF 40.4 ) Pub Date : 2024-09-13 , DOI: 10.1039/d4cs00420e
Xuelan Hou _{1,

2} , Yiyang Li ₂ , Hang Zhang ₃ , Peter D Lund ₃ , James Kwan ₁ , Shik Chi Edman Tsang ₂

Affiliation

Since its advent in 2011, black titanium oxide (B-TiO_x) has garnered significant attention due to its exceptional optical characteristics, notably its enhanced absorption spectrum ranging from 200 to 2000 nm, in stark contrast to its unmodified counterpart. The escalating urgency to address global climate change has spurred intensified research into this material for sustainable hydrogen production through thermal, photocatalytic, electrocatalytic, or hybrid water-splitting techniques. The rapid advancements in this dynamic field necessitate a comprehensive update. In this review, we endeavor to provide a detailed examination and forward-looking insights into the captivating attributes, synthesis methods, modifications, and characterizations of B-TiO_x, as well as a nuanced understanding of its physicochemical properties. We place particular emphasis on the potential integration of B-TiO_x into solar and electrochemical energy systems, highlighting its applications in green hydrogen generation, CO₂ reduction, and supercapacitor technology, among others. Recent breakthroughs in the structure–property relationship of B-TiO_x and its applications, grounded in both theoretical and empirical studies, are underscored. Additionally, we will address the challenges of scaling up B-TiO_x production, its long-term stability, and economic viability to align with ambitious future objectives.

中文翻译：

黑色氧化钛：合成、改性、表征、理化性质以及能源转换和储存以及环境可持续性的新兴应用

自 2011 年问世以来，黑色氧化钛（B-TiO_x）因其卓越的光学特性而备受关注，尤其是其增强的吸收光谱范围为 200 至 2000 nm，与未改性的同类产品形成鲜明对比。应对全球气候变化的紧迫性日益加剧，这促使人们加强对这种材料的研究，通过热、光催化、电催化或混合分解水技术实现可持续制氢。这个动态领域的快速发展需要全面更新。在这篇综述中，我们努力对 B-TiO_x 的迷人属性、合成方法、修饰和表征以及对其物理化学性质的细致理解提供详细的检查和前瞻性见解。我们特别强调 B-TiO_x 在太阳能和电化学能源系统中的潜力，重点介绍了其在绿色氢气生产、二氧化碳减排和超级电容器技术等方面的应用。强调了 B-TiO_x 的结构-性能关系及其应用的最新突破，这些突破基于理论和实证研究。此外，我们将应对扩大 B-TiO_x 生产、其长期稳定性和经济可行性的挑战，以符合雄心勃勃的未来目标。

更新日期：2024-09-13

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