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Oxygen-Stable Electrochemical CO2 Capture using Redox-Active Heterocyclic Benzodithiophene Quinone
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-09-09 , DOI: 10.1002/anie.202412229
Maryam Abdinejad 1 , Hyowon Seo 2 , Michael Edward Lev Massen-Hane 2 , T Alan Hatton 3
Affiliation  

CO2 capture was achieved with over 90 % capacity utilization in a 100-hour cycle using a heterocyclic benzodithiophene quinone in a flow system containing 13 % CO2 and 3.5 % O2, demonstrating its potential for real-world applications. This process was investigated through a combined experimental and computational approach to elucidate the kinetic and thermodynamic mechanisms underlying the carbon capture efficiency.

中文翻译:


使用氧化还原活性杂环苯并二噻吩醌进行氧稳定电化学 CO2 捕获



在含有 13 % CO2 和 3.5 % O2 的流动系统中,使用杂环苯并噻吩醌在 100 小时周期内以超过 90% 的容量利用率实现 CO2 捕获,展示了其实际应用的潜力。通过实验和计算相结合的方法研究了这一过程,以阐明碳捕获效率背后的动力学和热力学机制。
更新日期:2024-09-09
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