(2 + 2 + 1)-Cyclization of Glycine Derivatives with Alkenes and CO2,Organic Letters

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(2 + 2 + 1)-Cyclization of Glycine Derivatives with Alkenes and CO2
Organic Letters ( IF 4.9 ) Pub Date : 2024-09-05 , DOI: 10.1021/acs.orglett.4c02805
Youwan Ye ₁ , Congde Huo ₁

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A highly atom-economic (2 + 2 + 1)-cyclization of glycine derivatives with alkenes and CO₂ facilitated by visible light catalysis is described. A range of multisubstituted pyrrolidones were synthesized under simple and mild reaction conditions. A reasonable mechanism involving redox-neutral radical-polar crossover is proposed.

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