Cyclic Sulfoximines as Methyl and Perdeuteromethyl Transfer Agents and Their Applications in Photoredox Catalysis,Angewandte Chemie International Edition

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Cyclic Sulfoximines as Methyl and Perdeuteromethyl Transfer Agents and Their Applications in Photoredox Catalysis
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-09-05 , DOI: 10.1002/anie.202412418
Peng Wu ₁ , Gabriel Goujon ₂ , Shulei Pan ₁ , Béatrice Tuccio ₃ , Bruce Pégot ₂ , Guillaume Dagousset ₂ , Elsa Anselmi ₂ , Emmanuel Magnier ₂ , Carsten Bolm ₄

Affiliation

Under photoredox catalysis, novel heterocyclic sulfoximines serve as methyl and perdeuteromethyl radical sources. The reagents are bench-stable and easy-to-use. Various radical acceptors can be applied leading to products in good yields. Up-scaling has been achieved by using a photoflow reactor. Physicochemical studies suggest a photoredox process.

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