npj Quantum Materials ( IF 5.4 ) Pub Date : 2024-09-04 , DOI: 10.1038/s41535-024-00678-8 Hui-Ke Jin , Wilhelm Kadow , Michael Knap , Johannes Knolle
We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange K the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group simulations on finite systems, we uncover that the introduction of a single hole, corresponding to ≈1% hole doping for the system size we consider, with a hopping strength of just t ~ 0.28K is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic exchange Γ drives the polarization towards the [111] direction via a transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental implications for Kitaev candidate materials.
中文翻译:
空穴掺杂基塔耶夫自旋液体的动力学铁磁性和拓扑磁振子
我们研究了空穴掺杂对基塔耶夫自旋液体 (KSL) 的影响,发现对于铁磁 (FM) 基塔耶夫交换K ,系统非常容易形成 FM 自旋极化。通过有限系统上的密度矩阵重整化群模拟,我们发现单孔的引入,对应于我们考虑的系统尺寸的 ≈1% 孔掺杂,跳跃强度仅为t ~ 0.28 K就足以破坏分数化和由于有序-无序机制,使自旋沿 [001] 方向极化。考虑到与材料相关的 FM 各向异性交换Г通过过渡到具有手性磁振子激发的拓扑 FM 状态,将极化驱动到 [111] 方向。我们开发了一种结合费米子完整子和玻色磁子的部分子平均场理论,该理论解释了掺杂引起的调频相位和拓扑磁子激发。我们讨论了基塔耶夫候选材料的实验意义。