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Efficient Electrocatalytic Oxidation of Glycerol to Formate Coupled with Nitrate Reduction over Cu-Doped NiCo Alloy Supported on Nickel Foam
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-08-12 , DOI: 10.1002/anie.202411542 Chenyang Li 1 , Hao Li 1 , Bo Zhang 2 , Huan Li 1 , Yi Wang 1 , Xiao Wang 1 , Pratteek Das 3 , Yuejiao Li 1 , Xianhong Wu 4 , Yifan Li 5 , Yi Cui 5 , Jianping Xiao 1 , Zhong-Shuai Wu 6
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-08-12 , DOI: 10.1002/anie.202411542 Chenyang Li 1 , Hao Li 1 , Bo Zhang 2 , Huan Li 1 , Yi Wang 1 , Xiao Wang 1 , Pratteek Das 3 , Yuejiao Li 1 , Xianhong Wu 4 , Yifan Li 5 , Yi Cui 5 , Jianping Xiao 1 , Zhong-Shuai Wu 6
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A Cu doped NiCo alloy supported on nickel foam (Cu−NiCo/NF) is synthesized. Because Cu doping facilitates the coupling of reaction intermediates with surface adsorbed oxygen, the catalyst shows excellent catalytic activity and formate Faraday efficiency. Besides, a coupled system of glycerol oxidation with nitrate reduction is constructed, which further enhances the activity, reduces energy consumption and gains valuable ammonia simultaneously.
中文翻译：
在泡沫镍负载的 Cu 掺杂 NiCo 合金上实现甘油高效电催化氧化成甲酸盐耦合硝酸盐还原
合成了一种负载在泡沫镍上的 Cu 掺杂 NiCo 合金 （Cu-NiCo/NF）。由于 Cu 掺杂促进了反应中间体与表面吸附氧的偶联，因此催化剂表现出优异的催化活性和甲酸盐法拉第效率。此外，构建了甘油氧化与硝酸盐还原的耦合系统，进一步增强了活性，降低了能耗，同时获得了宝贵的氨。
更新日期：2024-08-12
中文翻译：
在泡沫镍负载的 Cu 掺杂 NiCo 合金上实现甘油高效电催化氧化成甲酸盐耦合硝酸盐还原
合成了一种负载在泡沫镍上的 Cu 掺杂 NiCo 合金 （Cu-NiCo/NF）。由于 Cu 掺杂促进了反应中间体与表面吸附氧的偶联，因此催化剂表现出优异的催化活性和甲酸盐法拉第效率。此外，构建了甘油氧化与硝酸盐还原的耦合系统，进一步增强了活性，降低了能耗，同时获得了宝贵的氨。
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