Leveraging Ion Pairing and Transport in Localized High-Concentration Electrolytes for Reversible Lithium Metal Anodes at Low Temperatures,Angewandte Chemie International Edition

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Leveraging Ion Pairing and Transport in Localized High-Concentration Electrolytes for Reversible Lithium Metal Anodes at Low Temperatures
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-07-20 , DOI: 10.1002/anie.202412239
Zhengfei Zhao ₁ , Aoxuan Wang ₁ , Aosai Chen ₂ , Yumeng Zhao ₁ , Zhenglin Hu ₁ , Kai Wu ₂ , Jiayan Luo ₃

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Along with the desolvation barrier, bulk transport properties also determine Li deposition behavior at ultra-low temperatures. The combination of moderately weak solvent and low viscosity diluent allows for low desolvation energy and high Li⁺ transference number while maintaining adequate ion conduction and diffusion. Therefore, exceptional Li metal Coulombic efficiency at extremely low temperatures is achieved.

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