Optical Review ( IF 1.1 ) Pub Date : 2024-07-12 , DOI: 10.1007/s10043-024-00899-z Narumi Asato , Ryushi Fujimura
The Ag semi-shell, a nanostructure comprising a dielectric nanosphere partially covered with Ag metal, can have its metallic shell deformed through a melting process under the illumination of plasmonic resonance. We have investigated the photothermal deformation process in Ag semi-shells and observed intensity-dependent melting deformation of the shell and a corresponding blueshift of the resonance peak. This indicates that the plasmonic resonance of the Ag semi-shells can be continuously controlled through laser irradiation. Furthermore, when the Ag semi-shells were coated with a UV-curable resin, the initial resonance peak wavelength was red-shifted, and the controllable spectral region was increased by a factor of two compared to that without the UV-curable resin. This large continuous control of the optical response through melting deformation of the shell has potential applications in optical memory, plasmonic color, and other areas.
中文翻译:
通过Ag-SiO2半壳纳米结构的光热变形实现可调谐等离子体共振以及通过紫外固化树脂扩大可控光谱区域
银半壳是一种由部分覆盖有银金属的介电纳米球组成的纳米结构,在等离子体共振照射下,其金属壳可以通过熔化过程而变形。我们研究了银半壳的光热变形过程,并观察到壳的强度依赖性熔化变形和相应的共振峰蓝移。这表明银半壳的等离子体共振可以通过激光照射连续控制。此外,当银半壳涂有紫外光固化树脂时,初始共振峰波长发生红移,可控光谱范围比没有紫外光固化树脂时增加了两倍。这种通过壳的熔化变形对光学响应进行大的连续控制在光学记忆、等离子体颜色和其他领域具有潜在的应用。