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Spin-Dependent ππ* Gap in Graphene on a Magnetic Substrate
Physical Review Letters ( IF 8.1 ) Pub Date : 2024-06-28 , DOI: 10.1103/physrevlett.132.266401
P. M. Sheverdyaeva 1 , G. Bihlmayer 2, 3 , E. Cappelluti 1 , D. Pacilé 4 , F. Mazzola 5, 6 , N. Atodiresei 2, 3 , M. Jugovac 7 , I. Grimaldi 4 , G. Contini 1 , Asish K. Kundu 1, 8, 9 , I. Vobornik 6 , J. Fujii 6 , P. Moras 1 , C. Carbone 1 , L. Ferrari 1
Affiliation  

We present a detailed analysis of the electronic properties of graphene/Eu/Ni(111). By using angle- and spin-resolved photoemission spectroscopy and ab initio calculations, we show that the intercalation of Eu in the graphene/Ni(111) interface gives rise to a gapped freestanding dispersion of the ππ* Dirac cones at the K¯ point with an additional lifting of the spin degeneracy due to the mixing of graphene and Eu states. The interaction with the magnetic substrate results in a large spin-dependent gap in the Dirac cones with a topological nature characterized by a large Berry curvature and a spin-polarized Van Hove singularity, whose closeness to the Fermi level gives rise to a polaronic band.

中文翻译:


磁性基底上石墨烯中自旋相关的 ππ* 能隙



我们对石墨烯/Eu/Ni(111) 的电子特性进行了详细分析。通过使用角度和自旋分辨光电子能谱以及从头计算,我们表明,Eu 在石墨烯/Ni(111) 界面中的插层会导致 ππ* 狄拉克锥体在 K¯ 点由于石墨烯和Eu态的混合而额外提升了自旋简并性。与磁性基底的相互作用导致狄拉克锥中存在较大的自旋相关间隙,其拓扑性质以大贝里曲率和自旋极化范霍夫奇点为特征,其接近费米能级产生极化子带。
更新日期:2024-06-29
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