Rational Design of Catalysts with Spinel Nanostructures for Thermal-Driven C1 Conversion,ACS Catalysis

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Rational Design of Catalysts with Spinel Nanostructures for Thermal-Driven C1 Conversion
ACS Catalysis ( IF 11.3 ) Pub Date : 2024-06-17 , DOI: 10.1021/acscatal.4c01138
Xiaoxue Han ₁ , Dan Guo _{1,

2} , Yong Wang ₁ , Shouying Huang _{1,

2} , Mei-Yan Wang _{1,

2} , Yue Wang _{1,

3} , Maoshuai Li _{1,

3} , Shengping Wang ₁ , Xinbin Ma ₁

Affiliation

The oriented conversion of C1 molecules including CO, CO₂, CH₄, and CH₃OH has received great attention in the past few decades because of its essential role in sustainable chemistry. Spinel oxides with fine hardness, great thermal stability, and tunable chemical properties are advantageous catalysts or precursors in the activation of inert C1 molecules for the production of high-value-added chemicals. This review provides a thorough overview of the recent developments in spinel-structured nanocatalysts for the processes of thermal-driven C1 conversion, highlighting the spinel-structured advantages in deriving active metals, stabilizing metal cations, constructing adjacent synergic sites, and tuning oxygen vacancies. Finally, the potential challenges and development directions are discussed for the application of spinel-structured catalysts in thermal-driven C1 conversion reactions.

中文翻译：

热驱动 C1 转化尖晶石纳米结构催化剂的合理设计

CO、CO ₂ 、CH ₄ 和 CH ₃ OH 等 C1 分子的定向转化由于其本质特征在过去几十年中受到了极大的关注。在可持续化学中的作用。尖晶石氧化物具有良好的硬度、良好的热稳定性和可调节的化学性质，是活化惰性 C1 分子以生产高附加值化学品的有利催化剂或前体。本综述全面概述了尖晶石结构纳米催化剂在热驱动 C1 转化过程中的最新进展，强调了尖晶石结构在衍生活性金属、稳定金属阳离子、构建相邻协同位点和调节氧空位方面的优势。最后，讨论了尖晶石结构催化剂在热驱动C1转化反应中应用的潜在挑战和发展方向。

更新日期：2024-06-17

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