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Atomic-scale visualization of a cascade of magnetic orders in the layered antiferromagnet GdTe3
npj Quantum Materials ( IF 5.4 ) Pub Date : 2024-06-01 , DOI: 10.1038/s41535-024-00660-4
Arjun Raghavan , Marisa Romanelli , Julian May-Mann , Anuva Aishwarya , Leena Aggarwal , Anisha G. Singh , Maja D. Bachmann , Leslie M. Schoop , Eduardo Fradkin , Ian R. Fisher , Vidya Madhavan

GdTe3 is a layered antiferromagnet which has attracted attention due to its exceptionally high mobility, distinctive unidirectional incommensurate charge density wave (CDW), superconductivity under pressure, and a cascade of magnetic transitions between 7 and 12 K, with as yet unknown order parameters. Here, we use spin-polarized scanning tunneling microscopy to directly image the charge and magnetic orders in GdTe3. Below 7 K, we find a striped antiferromagnetic phase with twice the periodicity of the Gd lattice and perpendicular to the CDW. As we heat the sample, we discover a spin density wave with the same periodicity as the CDW between 7 and 12 K; the viability of this phase is supported by our Landau free energy model. Our work reveals the order parameters of the magnetic phases in GdTe3 and shows how the interplay between charge and spin can generate a cascade of magnetic orders.



中文翻译:


层状反铁磁体 GdTe3 中一系列磁序的原子尺度可视化



GdTe 3 是一种层状反铁磁体,由于其极高的迁移率、独特的单向不通约电荷密度波 (CDW)、压力下的超导性以及 7 至 12 K 之间的级联磁转变而引起了人们的关注,尚不清楚订单参数。在这里,我们使用自旋偏振扫描隧道显微镜直接对 GdTe 3 中的电荷和磁序进行成像。在 7 K 以下,我们发现了条状反铁磁相,其周期性是 Gd 晶格的两倍,并且垂直于 CDW。当我们加热样品时,我们发现自旋密度波在 7 到 12 K 之间具有与 CDW 相同的周期;我们的朗道自由能模型支持了这一阶段的可行性。我们的工作揭示了 GdTe 3 中磁相的有序参数,并展示了电荷和自旋之间的相互作用如何产生一系列磁序。

更新日期:2024-06-02
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