Silica-Derived Nanostructured Electrode Materials for ORR, OER, HER, CO2RR Electrocatalysis, and Energy Storage Applications: A Review**,The Chemical Record

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Silica-Derived Nanostructured Electrode Materials for ORR, OER, HER, CO2RR Electrocatalysis, and Energy Storage Applications: A Review**
The Chemical Record ( IF 7.0 ) Pub Date : 2024-03-26 , DOI: 10.1002/tcr.202300234
Sammy Onajah _{1,

2} , Rajib Sarkar ₃ , Md Shafiul Islam ₁ , Marja Lalley ₄ , Kishwar Khan ₅ , Muslum Demir _{6,

7} , Hani Nasser Abdelhamid _{8,

9} , Ahmed A Farghaly _{1,

2,

10}

Affiliation

Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, Illinois, 60439, United States.
Pritzker School of Molecular Engineering, The University of Chicago, Chicago, Illinois, 60637, United States.
Department of Chemistry, Virginia Commonwealth University, Richmond, Virginia, 23284-2006, United States.
Department of Chemistry, University of Chicago, Chicago, Illinois, 60637, United States.
Department of Chemistry, City University of Hong Kong, Hong Kong, 999077, China.
Department of Chemical Engineering, Bogazici University, 34342, Istanbul, Turkey.
TUBITAK Marmara Research Center, Material Institute, Gebze, 41470, Turkey.
Advanced Multifunctional Materials Laboratory, Department of Chemistry, Assiut University, Assiut, 71516, Egypt.
Egyptian Russian University, Badr City, Cairo, 11829, Egypt.
Chemistry Department, Faculty of Science, Assiut University, Assiut, 71516, Egypt.

Silica-derived nanostructured catalysts (SDNCs) are a class of materials synthesized using nanocasting and templating techniques, which involve the sacrificial removal of a silica template to generate highly porous nanostructured materials. The surface of these nanostructures is functionalized with a variety of electrocatalytically active metal and non-metal atoms. SDNCs have attracted considerable attention due to their unique physicochemical properties, tunable electronic configuration, and microstructure. These properties make them highly efficient catalysts and promising electrode materials for next generation electrocatalysis, energy conversion, and energy storage technologies. The continued development of SDNCs is likely to lead to new and improved electrocatalysts and electrode materials. This review article provides a comprehensive overview of the recent advances in the development of SDNCs for electrocatalysis and energy storage applications. It analyzes 337,061 research articles published in the Web of Science (WoS) database up to December 2022 using the keywords “silica”, “electrocatalysts”, “ORR”, “OER”, “HER”, “HOR”, “CO₂RR”, “batteries”, and “supercapacitors”. The review discusses the application of SDNCs for oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), carbon dioxide reduction reaction (CO₂RR), supercapacitors, lithium-ion batteries, and thermal energy storage applications. It concludes by discussing the advantages and limitations of SDNCs for energy applications.

中文翻译：

用于 ORR、OER、HER、CO2RR 电催化和储能应用的二氧化硅衍生纳米结构电极材料：综述**

二氧化硅衍生的纳米结构催化剂（SDNC）是一类使用纳米铸造和模板技术合成的材料，其中涉及牺牲二氧化硅模板的去除以生成高度多孔的纳米结构材料。这些纳米结构的表面被各种电催化活性金属和非金属原子功能化。 SDNC由于其独特的物理化学性质、可调节的电子构型和微观结构而引起了广泛的关注。这些特性使它们成为高效催化剂和用于下一代电催化、能量转换和能量存储技术的有前景的电极材料。 SDNC 的持续发展可能会带来新的和改进的电催化剂和电极材料。这篇综述文章全面概述了用于电催化和储能应用的 SDNC 开发的最新进展。它分析了截至 2022 年 12 月在 Web of Science (WoS) 数据库中发表的 337,061 篇研究文章，使用关键词“silica”、“electriccatalysts”、“ORR”、“OER”、“HER”、“HOR”、“CO ₂ RR” ”、“电池”和“超级电容器”。该综述讨论了SDNCs在氧还原反应(ORR)、析氧反应(OER)、析氢反应(HER)、二氧化碳还原反应(CO ₂ RR)、超级电容器、锂离子电池和热能储存方面的应用应用程序。最后讨论了 SDNC 在能源应用中的优势和局限性。

更新日期：2024-03-26

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