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Rational Design of an In-Situ Polymer-Inorganic Hybrid Solid Electrolyte Interphase for Realising Stable Zn Metal Anode under Harsh Conditions
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-03-25 , DOI: 10.1002/anie.202401987
Ruwei Chen 1, 2 , Wei Zhang 1 , Chaohong Guan 3 , Yundong Zhou 4 , Ian Gilmore 4 , Hao Tang 2 , Zhenyu Zhang 5 , Haobo Dong 1 , Yuhang Dai 1 , Zijuan Du 1 , Xuan Gao 1 , Wei Zong 1 , Yewei Xu 1 , Peie Jiang 1 , Jiyang Liu 1 , Fangjia Zhao 1 , Jianwei Li 1 , Xiaohui Wang 2 , Guanjie He 1
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-03-25 , DOI: 10.1002/anie.202401987
Ruwei Chen 1, 2 , Wei Zhang 1 , Chaohong Guan 3 , Yundong Zhou 4 , Ian Gilmore 4 , Hao Tang 2 , Zhenyu Zhang 5 , Haobo Dong 1 , Yuhang Dai 1 , Zijuan Du 1 , Xuan Gao 1 , Wei Zong 1 , Yewei Xu 1 , Peie Jiang 1 , Jiyang Liu 1 , Fangjia Zhao 1 , Jianwei Li 1 , Xiaohui Wang 2 , Guanjie He 1
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A robust polymer-inorganic SEI is in situ constructed on Zn anode through controllable polymerization and coprecipitation mechanism. Compared with bare Zn and recent in situ SEIs, polymer-inorganic SEI combines both superiorities of polymer phases for high toughness and inorganic phases for high modulus, enabling stable electrode/electrolyte interface even under harsh conditions.
中文翻译：
原位聚合物-无机杂化固体电解质界面的合理设计，实现恶劣条件下稳定的锌金属负极
通过可控聚合和共沉淀机制，在 Zn 负极上原位构建了坚固的聚合物-无机 SEI。与裸锌和最新的原位 SEI 相比，聚合物-无机 SEI 结合了聚合物相的高韧性和高模量的无机相的优点，即使在恶劣条件下也能实现稳定的电极/电解质界面。
更新日期：2024-03-25
中文翻译：
原位聚合物-无机杂化固体电解质界面的合理设计，实现恶劣条件下稳定的锌金属负极
通过可控聚合和共沉淀机制，在 Zn 负极上原位构建了坚固的聚合物-无机 SEI。与裸锌和最新的原位 SEI 相比，聚合物-无机 SEI 结合了聚合物相的高韧性和高模量的无机相的优点，即使在恶劣条件下也能实现稳定的电极/电解质界面。
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