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Simple Functionalization of a Donor Monomer to Enhance Charge Transfer in Porous Polymer Networks for Photocatalytic Hydrogen Evolution
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-02-14 , DOI: 10.1002/anie.202319395
Jiwon Kim 1 , Jong-Pil Jeon 1 , Young Hyun Kim 1 , Nguyen Thi Dieu Anh 2 , Kunook Chung 2, 3 , Jeong-Min Seo 1 , Jong-Beom Baek 1
Affiliation  

Triazatruxene (TAT)-based PPNs were synthesized to investigate how the existence of a hexyl functional group would affect charge transfer. The hexyl group on the TAT unit ensured the transfer of photoexcited electrons from a donor unit to an acceptor unit, resulting in improved photocatalytic activity and hydrogen production.

中文翻译:


供体单体的简单功能化可增强多孔聚合物网络中的电荷转移以实现光催化析氢



合成了基于三氮杂苯 (TAT) 的 PPN,以研究己基官能团的存在如何影响电荷转移。 TAT单元上的己基确保光激发电子从供体单元转移到受体单元,从而提高光催化活性和氢气产量。
更新日期:2024-02-14
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