<br>丹尼尔电池万岁：从电冶金到电化学储能,Advanced Functional Materials

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丹尼尔电池万岁：从电冶金到电化学储能
Advanced Functional Materials ( IF 18.5 ) Pub Date : 2024-02-12 , DOI: 10.1002/adfm.202400289
Hongyan Yuan ₁ , Jingyi Luan ₁ , Jie Liu ₁ , Cheng Zhong _{1,

2}

Affiliation

Daniell电池是第一个投入实际应用的电池，被认为是电冶金的第一次实践，是连接电冶金和电化学储能的桥梁。尽管丹尼尔电池后来因不可充电的特性和自放电副反应而被其他电池所取代，但受丹尼尔电池启发的基于沉积/溶解机制的电极的研究却从未停止过，因为它与普通电池相比具有无可比拟的优势。基于离子嵌入/脱出机理和固相氧化还原反应机理的电极。近年来，沉积/溶解电池（DDB）的研究受到越来越多的关注，其中两种沉积/溶解化学耦合。本文简要介绍了DDB从电冶金的起源到储能电池的发现的演变过程。此外，系统分析了两种主要类型的DDB，包括Pb基DDB和Mn基DDB，并概述和深入讨论了关键问题和解决方案。最后，对未来的研究方向提出了个人的看法，旨在为DDB的性能提升和实际应用提供指导。

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Hail to Daniell Cell: From Electrometallurgy to Electrochemical Energy Storage

Daniell cell is the first battery to be used in practice and is considered to be the first practice of electrometallurgy, which is the bridge connecting electrometallurgy and electrochemical energy storage. Although Daniell cell is later replaced by other batteries due to the unrechargeable characteristic and the self-discharge side reaction, the research on the electrode based on the deposition/dissolution mechanism inspired by Daniell cell has never been stopped due to its incomparable advantages compared with the electrodes based on the ion insertion/extraction mechanism and the solid-phase redox reaction mechanism. In recent years, increased focus has been placed on the research of deposition/dissolution battery (DDB), in which two deposition/dissolution chemistries are coupled. In this review, the evolution process from the origin of electrometallurgy to the discovery of energy storage batteries of DDBs is briefly introduced. Furthermore, two main types of DDBs, including Pb-based DDBs and Mn-based DDBs, are analyzed systematically, and the critical issues and solutions are outlined and discussed in depth. Finally, personal perspectives on the future research directions are highlighted, aiming to provide guidance for performance improvement and the practical application of DDBs.

更新日期：2024-02-12

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