Dual-Salt Electrolyte Additive Enables High Moisture Tolerance and Favorable Electric Double Layer for Lithium Metal Battery,Angewandte Chemie International Edition

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Dual-Salt Electrolyte Additive Enables High Moisture Tolerance and Favorable Electric Double Layer for Lithium Metal Battery
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2024-02-02 , DOI: 10.1002/anie.202314876
Zuxin Wen ₁ , Wenqiang Fang ₁ , Fenglin Wang ₁ , Hong Kang ₁ , Shuoqing Zhao ₂ , Shaojun Guo ₂ , Gen Chen ₁

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A dual-salt additive-reinforced carbonate electrolyte (LTFAN) is proposed for stabilizing high-voltage LMBs. The in situ generated nitrogenous and fluoride-rich electrode electrolyte interphase with LTFAN vastly accelerates the interfacial reaction dynamics, and dual-salt additive notably strengthens the moisture tolerance. A thermodynamically favorable electric double layer at charged cathode interface is constructed.

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