当前位置：
X-MOL 学术
›
J. Colloid Interface Sci.
›
论文详情
Our official English website, www.x-mol.net, welcomes your
feedback! (Note: you will need to create a separate account there.)
MOF-based/derived catalysts for electrochemical overall water splitting
Journal of Colloid and Interface Science ( IF 9.4 ) Pub Date : 2024-01-19 , DOI: 10.1016/j.jcis.2024.01.106 Yujia He 1 , Wei Liu 2 , Jingquan Liu 3
Journal of Colloid and Interface Science ( IF 9.4 ) Pub Date : 2024-01-19 , DOI: 10.1016/j.jcis.2024.01.106 Yujia He 1 , Wei Liu 2 , Jingquan Liu 3
Affiliation
|
Water-splitting electrocatalysis has gained increasing attention as a promising strategy for developing renewable energy in recent years, but its high overpotential caused by the unfavorable thermodynamics has limited its widespread implementation. Therefore, there is an urgent need to design catalytic materials with outstanding activity and stability that can overcome the high overpotential and thus improve the electrocatalytic efficiency. Metal-organic frameworks (MOFs) based and/or derived materials are widely used as water-splitting catalysts because of their easily controlled structures, abundant heterointerfaces and increased specific surface area. Herein, some recent research findings on MOFs-based/derived materials are summarized and presented. First, the mechanism and evaluation parameters of electrochemical water splitting are described. Subsequently, advanced modulation strategies for designing MOFs-based/derived catalysts and their catalytic performance toward water splitting are summarized. In particular, the correlation between chemical composition/structural functionalization and catalytic performance is highlighted. Finally, the future outlook and challenges for MOFs materials are also addressed.
中文翻译：
用于电化学整体水分解的 MOF 基/衍生催化剂
近年来，水分解电催化作为开发可再生能源的一种有前景的策略受到越来越多的关注，但其不利的热力学导致的高过电势限制了其广泛应用。因此，迫切需要设计具有优异活性和稳定性的催化材料，能够克服高过电势，从而提高电催化效率。基于金属有机框架（MOF）和/或衍生材料因其易于控制的结构、丰富的异质界面和增加的比表面积而被广泛用作水分解催化剂。本文总结并介绍了有关 MOF 基/衍生材料的一些最新研究成果。首先，描述了电化学水分解的机理和评价参数。随后，总结了设计 MOF 基/衍生催化剂的先进调制策略及其对水分解的催化性能。特别强调了化学成分/结构功能化与催化性能之间的相关性。最后，还讨论了 MOF 材料的未来前景和挑战。
更新日期：2024-01-19
中文翻译：
用于电化学整体水分解的 MOF 基/衍生催化剂
近年来，水分解电催化作为开发可再生能源的一种有前景的策略受到越来越多的关注，但其不利的热力学导致的高过电势限制了其广泛应用。因此，迫切需要设计具有优异活性和稳定性的催化材料，能够克服高过电势，从而提高电催化效率。基于金属有机框架（MOF）和/或衍生材料因其易于控制的结构、丰富的异质界面和增加的比表面积而被广泛用作水分解催化剂。本文总结并介绍了有关 MOF 基/衍生材料的一些最新研究成果。首先，描述了电化学水分解的机理和评价参数。随后，总结了设计 MOF 基/衍生催化剂的先进调制策略及其对水分解的催化性能。特别强调了化学成分/结构功能化与催化性能之间的相关性。最后，还讨论了 MOF 材料的未来前景和挑战。
京公网安备 11010802027423号