Exploring the Cation Regulation Mechanism for Interfacial Water Involved in the Hydrogen Evolution Reaction by In Situ Raman Spectroscopy,Nano-Micro Letters

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Exploring the Cation Regulation Mechanism for Interfacial Water Involved in the Hydrogen Evolution Reaction by In Situ Raman Spectroscopy
Nano-Micro Letters ( IF 31.6 ) Pub Date : 2023-12-18 , DOI: 10.1007/s40820-023-01285-1
Xueqiu You ₁ , Dongao Zhang ₂ , Xia-Guang Zhang ₃ , Xiangyu Li ₁ , Jing-Hua Tian ₄ , Yao-Hui Wang ₂ , Jian-Feng Li _{2,

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Affiliation

In situ Raman spectroscopy study of the cation regulation for interfacial water on Au@Pd core–shell nanoparticle surface during hydrogen evolution reaction process.
Direct spectral evidence reveals new strategies to optimize the structure of interfacial water by the adjusting of radius and valence of the cation in the electrolyte.
The optimized structure of interfacial water will improve the charge transfer efficiency between the water and electrode increasing the performance of the hydrogen evolution reaction.

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