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Stabilizing Sulfur Sites in Tetraoxygen Tetrahedral Coordination Structure for Efficient Electrochemical Water Oxidation
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-12-07 , DOI: 10.1002/anie.202313185
Jing Jin 1 , Jie Yin 1 , Yang Hu 1 , Yao Zheng 2 , Hongbo Liu 1 , Xinyao Wang 1 , Pinxian Xi 1 , Chun-Hua Yan 1, 3
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-12-07 , DOI: 10.1002/anie.202313185
Jing Jin 1 , Jie Yin 1 , Yang Hu 1 , Yao Zheng 2 , Hongbo Liu 1 , Xinyao Wang 1 , Pinxian Xi 1 , Chun-Hua Yan 1, 3
Affiliation
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The tetraoxygen tetrahedral coordination structure (S-O4) inside NiO is produced by encapsulating S atoms at the tetrahedral sites of the NaCl-type oxide. This unique structure could trigger a S-promoted lattice-oxygen-mediated mechanism (SLOM) during the oxygen evolution reaction (OER), which greatly elevated the catalytic performance.
中文翻译:
稳定四氧四面体配位结构中的硫位点以实现高效电化学水氧化
NiO内部的四氧四面体配位结构(SO 4 )是通过将S原子封装在NaCl型氧化物的四面体位点而产生的。这种独特的结构可以在析氧反应(OER)过程中触发S促进的晶格氧介导机制(SLOM),从而大大提高催化性能。
更新日期:2023-12-07
中文翻译:
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稳定四氧四面体配位结构中的硫位点以实现高效电化学水氧化
NiO内部的四氧四面体配位结构(SO 4 )是通过将S原子封装在NaCl型氧化物的四面体位点而产生的。这种独特的结构可以在析氧反应(OER)过程中触发S促进的晶格氧介导机制(SLOM),从而大大提高催化性能。