Lamellar Crystal Structure and Haldane Magnetism in NH4VPO4OH,Angewandte Chemie International Edition

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Lamellar Crystal Structure and Haldane Magnetism in NH4VPO4OH
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-12-06 , DOI: 10.1002/anie.202316719
Aleksandr Sh Samarin ₁ , Ivan A Trussov ₁ , Zlata V Pchelkina _{2,

3} , Stanislav S Fedotov ₁ , Yevgeniy A Ovchenkov _{4,

5} , Sergei V Zhurenko ₆ , Alexei V Tkachev ₆ , Andrei A Gippius ₅ , Larisa V Shvanskaya _{4,

5} , Alexander N Vasiliev _{4,

5}

Affiliation

A new compound, NH₄VPO₄OH, has been synthesized under mild hydrothermal condition. It possesses a lamellar crystal structure and shows a spin gap behavior inherent for the Haldane system. This rare ground state has been supported in the first-principles calculations.

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