Breaking Surface Atomic Monogeneity of Rh2P Nanocatalysts by Defect-Derived Phosphorus Vacancies for Efficient Alkaline Hydrogen Oxidation,Angewandte Chemie International Edition

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Breaking Surface Atomic Monogeneity of Rh2P Nanocatalysts by Defect-Derived Phosphorus Vacancies for Efficient Alkaline Hydrogen Oxidation
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-11-13 , DOI: 10.1002/anie.202315752
Hongpu Huang ₁ , Kai Liu ₁ , Fulin Yang ₂ , Junlin Cai ₁ , Shupeng Wang ₁ , Weizhen Chen ₁ , Qiuxiang Wang ₁ , Luhong Fu ₁ , Zhaoxiong Xie ₃ , Shuifen Xie ₁

Affiliation

Defect-derived surface phosphorus vacancies on ultrathin Rh₂P nanowires break the monogeneity and atomic regularity of thermodynamically stable P-terminated surfaces, which can create additional Rh sites to act as exclusive H adsorption sites and diminish the inhibition effect of the interfacial water network to achieve drastically improved alkaline HOR electrocatalysis.

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