Revealing the CO2 Conversion at Electrode/Electrolyte Interfaces in Li–CO2 Batteries via Nanoscale Visualization Methods,Angewandte Chemie International Edition

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Revealing the CO2 Conversion at Electrode/Electrolyte Interfaces in Li–CO2 Batteries via Nanoscale Visualization Methods
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-11-13 , DOI: 10.1002/anie.202316781
Zhen-Zhen Shen ₁ , Shuang-Yan Lang ₂ , Rui-Zhi Liu _{1,

3} , Chi Zhou ₁ , Yao-Zu Zhang _{1,

3} , Bing Liu _{3,

4} , Rui Wen _{1,

3}

Affiliation

Using in situ atomic force microscopy, laser confocal microscopy-differential interference contrast microscopy and Raman spectroscopy, we explored the electrode/electrolyte interfacial evolution in Li–CO₂ batteries. The results indicate that the laser alters the reaction pathways of the CO₂ reduction processes, which changes the morphological evolution of the discharge products at the interfaces, and in turn, affects the cell performance.

中文翻译：

通过纳米级可视化方法揭示 Li-CO2 电池中电极/电解质界面的 CO2 转化

利用原位原子力显微镜、激光共焦显微镜-微分干涉显微镜和拉曼光谱，我们探索了Li-CO ₂电池中电极/电解质界面的演化。结果表明，激光改变了CO ₂还原过程的反应路径，从而改变了界面处放电产物的形态演化，进而影响了电池性能。

更新日期：2023-11-13

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