<br>电化学二氧化碳转化为多碳的最新进展：从基础到工业化,Advanced Energy Materials

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电化学二氧化碳转化为多碳的最新进展：从基础到工业化
Advanced Energy Materials ( IF 24.4 ) Pub Date : 2023-11-02 , DOI: 10.1002/aenm.202302382
Changli Wang ₁ , Zunhang Lv ₁ , Xiao Feng ₁ , Wenxiu Yang ₁ , Bo Wang ₁

Affiliation

具有更高价值的电化学CO ₂ （eCO ₂ ）转化为多碳被认为是促进工业生产转型和碳循环绿色平衡的潜在途径。近年来，eCO ₂ 向多碳转化的进展取得了一系列进展，包括耦合机制的深入探索、表征技术的最新发展以及催化剂和电解系统的新颖跨学科设计策略。因此，有必要系统地概述eCO ₂ 从基础到工业化的多碳转化，以弥补已报道的有限和不充分的评论。为了填补上述研究空白，本综述重点关注 eCO ₂ 到多碳从基础到工业化的转化。首先，按照 eCO ₂ 还原、小分子偶联 eCO ₂ 还原的顺序总结了 eCO ₂ 向多碳转化的可能催化机制。，和eCO ₂ 串联转换。其次，介绍了有助于耦合机制合理化的最新原位表征技术。第三，简要分类了催化剂和电解系统的优化策略，以推动工业化进程。最后，合理提出了eCO ₂ 向多碳转化进一步发展的挑战和前景，旨在为该领域的后续工作提供启示。

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Recent Advances in Electrochemical CO2-to-Multicarbon Conversion: From Fundamentals to Industrialization

The electrochemical CO₂ (eCO₂)-to-multicarbon conversion with higher value is regarded as a potential way to promote the transformation of industrial production and the green balance of carbon cycle. Recently, a series of advances have been achieved in the progress of eCO₂-to-multicarbon conversion, including the in-depth exploration of coupling mechanisms, the up-to-date development of characterization techniques, and the novel interdisciplinary design strategies of catalysts and electrolytic systems. Therefore, it is essential to systematically overview the eCO₂-to-multicarbon conversion from fundamentals to industrialization, compensating for the limited and insufficient reviews that have been reported. To fill the aforementioned research gap, this overview is focused on the eCO₂-to-multicarbon conversion from fundamentals to industrialization. First, the possible catalytic mechanisms for eCO₂-to-multicarbon conversion are accordingly summarized in the order of eCO₂ reduction, small molecule-coupled eCO₂ reduction, and eCO₂ tandem conversion. Second, the up-to-date in situ characterization technologies assisting the rationalization of coupling mechanisms are presented. Third, the optimizing strategies of catalysts and electrolytic systems are briefly classified for the advance of industrialization process. Finally, challenges and perspectives for the further development of eCO₂-to-multicarbon conversion are reasonably proposed, aiming to offer insights for the following work in this field.

更新日期：2023-11-02

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