N,O-Codoped Onion-like Carbon Catalyzed Selective Oxidation of Methanol to Dimethoxymethane: Structure-Activity Relationship,ChemCatChem

当前位置： X-MOL 学术 › ChemCatChem › 论文详情

Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)

N,O-Codoped Onion-like Carbon Catalyzed Selective Oxidation of Methanol to Dimethoxymethane: Structure-Activity Relationship
ChemCatChem ( IF 3.8 ) Pub Date : 2023-10-26 , DOI: 10.1002/cctc.202300813
Yunli Bai ₁ , Xueya Dai ₂ , Tianlong Cao ₂ , Wei Qi ₃

Affiliation

Nitrogen, oxygen codoped onion-like carbon exhibits relatively high dimethoxymethane (DMM) selectivity from methanol at low reaction temperature (150 °C). The present research does not only demonstrate that nanocarbon is a promising catalyst for one-step synthesis of DMM but also highlights the key to increase the selectivity of DMM is to balance the redox and acidity of carbon catalysts.

中文翻译：

N,O-共掺杂洋葱状碳催化甲醇选择性氧化生成二甲氧基甲烷：构效关系

氮、氧共掺杂洋葱状碳在低反应温度（150 °C）下对甲醇表现出相对较高的二甲氧基甲烷（DMM）选择性。目前的研究不仅证明纳米碳是一种有前途的一步合成DMM的催化剂，而且强调了提高DMM选择性的关键是平衡碳催化剂的氧化还原性和酸性。

更新日期：2023-10-26

点击分享查看原文

点击收藏

阅读更多本刊新发论文本刊介绍/投稿指南