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Ferroelectric control of half-metallicity in A-type antiferromagnetic GdI2 bilayer coupled with ferroelectric In2Se3
Physica E: Low-dimensional Systems and Nanostructures ( IF 2.9 ) Pub Date : 2023-10-17 , DOI: 10.1016/j.physe.2023.115836
Kai Zhang , Xiaocha Wang , Wenbo Mi

A-type antiferromagnetic half-metal has great application potential in memory and spintronic devices. GdI2 bilayer is an A-type antiferromagnet with intralayer ferromagnetic coupling and interlayer antiferromagnetic coupling. Under an electric field, the spin degeneracy of the GdI2 bilayer is broken. As an electric field exceeds the critical electric field of 0.08 V/Å, the GdI2 bilayer exhibits antiferromagnetic half-metallicity. The bi-GdI2/In2Se3 heterojunction achieves the transition for GdI2 bilayer from semiconductor to half-metal and the ferroelectric memory can be achieved. The In2Se3/bi-GdI2/In2Se3 heterojunction realizes the switching of the spin direction of the half-metal for GdI2 bilayer and the spin field effect transistors can be achieved. The bi-GdI2/bi-In2Se3 heterojunction achieves functions similar to the bi-GdI2/In2Se3 heterojunction. The band transition mechanism of these heterojunctions is mainly caused by the charge transfer at the GdI2 and In2Se3 interfaces and the polarization field of In2Se3. The construction of heterojunction and biaxial strain can significantly regulate the magnetic anisotropy energy (MAE). The tensile strain increases the total MAE, while the compressive strain decreases the total MAE. The heterojunctions under biaxial strain always keep the easy magnetization axis in the xy plane. Based on the GdI2 bilayer, applying an electric field or constructing a van der Waals heterojunction can achieve antiferromagnetic half-metal.



中文翻译:

与铁电 In2Se3 耦合的 A 型反铁磁 GdI2 双层中半金属性的铁电控制

A型反铁磁半金属在存储器和自旋电子器件中具有巨大的应用潜力。GdI 2双层是一种具有层内铁磁耦合和层间反铁磁耦合的A型反铁磁体。在电场作用下,GdI 2双层的自旋简并性被破坏。当电场超过0.08 V/Å的临界电场时,GdI 2双层表现出反铁磁半金属性。bi-GdI 2 /In 2 Se 3异质结实现了GdI 2双层从半导体到半金属的转变,从而实现了铁电存储器。In 2 Se 3 /bi-GdI 2 /In 2 Se 3异质结实现了GdI 2双层半金属自旋方向的切换,可以实现自旋场效应晶体管。bi-GdI 2 /bi-In 2 Se 3异质结实现了与bi-GdI 2 /In 2 Se 3异质结类似的功能。这些异质结的能带跃迁机制主要是由GdI 2和In 2 Se 3界面处的电荷转移以及In 2 Se 3的极化场引起的。异质结和双轴应变的构建可以显着调节磁各向异性能量(MAE)。拉伸应变增加了总 MAE,而压缩应变则减少了总 MAE。双轴应变下的异质结始终将易磁化轴保持在xy平面内。基于GdI 2双层,施加电场或构建范德华异质结可以实现反铁磁半金属。

更新日期:2023-10-21
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