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Accelerating Ethanol Complete Electrooxidation via Introducing Ethylene as the Precursor for the C−C Bond Splitting
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-08-07 , DOI: 10.1002/anie.202308057
Teng Chen 1, 2 , Shen Xu 3 , Taotao Zhao 2 , Xiaohang Zhou 1 , Jianqiang Hu 1 , Xin Xu 1 , Chenjia Liang 2 , Min Liu 4 , Weiping Ding 2
Affiliation  

A unique ethylene-mediated pathway with a 100 % C1-selectivity for ethanol oxidation reaction (EOR) is proposed for the first time based on a well-structured Pt/Al2O3@TiAl catalyst, in which Al2O3 is responsible for generating ethylene from ethanol dehydration while Pt boosts the complete oxidation of ethylene to CO2.

中文翻译:

通过引入乙烯作为 C−C 键裂解前驱体加速乙醇完全电氧化

首次基于结构良好的 Pt/Al 2 O 3 @TiAl 催化剂(其中 Al 2 O 3 负责)提出了一种具有 100 % C1 选择性的独特乙烯介导乙醇氧化反应( EOR )途径用于从乙醇脱水生成乙烯,而Pt则促进乙烯完全氧化为CO 2
更新日期:2023-08-07
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