当前位置: X-MOL 学术Nat. Commun. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Ultrafast imaging of polariton propagation and interactions
Nature Communications ( IF 14.7 ) Pub Date : 2023-06-30 , DOI: 10.1038/s41467-023-39550-x
Ding Xu 1 , Arkajit Mandal 1 , James M Baxter 1 , Shan-Wen Cheng 1 , Inki Lee 1 , Haowen Su 1 , Song Liu 2 , David R Reichman 1 , Milan Delor 1
Affiliation  

Semiconductor excitations can hybridize with cavity photons to form exciton-polaritons (EPs) with remarkable properties, including light-like energy flow combined with matter-like interactions. To fully harness these properties, EPs must retain ballistic, coherent transport despite matter-mediated interactions with lattice phonons. Here we develop a nonlinear momentum-resolved optical approach that directly images EPs in real space on femtosecond scales in a range of polaritonic architectures. We focus our analysis on EP propagation in layered halide perovskite microcavities. We reveal that EP–phonon interactions lead to a large renormalization of EP velocities at high excitonic fractions at room temperature. Despite these strong EP–phonon interactions, ballistic transport is maintained for up to half-exciton EPs, in agreement with quantum simulations of dynamic disorder shielding through light-matter hybridization. Above 50% excitonic character, rapid decoherence leads to diffusive transport. Our work provides a general framework to precisely balance EP coherence, velocity, and nonlinear interactions.



中文翻译:

极化子传播和相互作用的超快成像

半导体激发可以与腔光子杂交形成具有卓越特性的激子极化子(EP),包括类光能量流与类物质相互作用相结合。为了充分利用这些特性,尽管存在物质介导的与晶格声子的相互作用,EP 仍必须保持弹道、相干的传输。在这里,我们开发了一种非线性动量分辨光学方法,可以在一系列极化子结构中以飞秒尺度直接对真实空间中的 EP 进行成像。我们重点分析层状卤化物钙钛矿微腔中的 EP 传播。我们揭示了 EP-声子相互作用导致室温下高激子分数下 EP 速度的大幅重正化。尽管有这些强烈的 EP-声子相互作用,弹道输运仍可维持高达半激子 EP,与通过光-物质杂交进行动态无序屏蔽的量子模拟一致。激子特性超过 50% 时,快速退相干会导致扩散传输。我们的工作提供了一个精确平衡 EP 相干性、速度和非线性相互作用的通用框架。

更新日期:2023-06-30
down
wechat
bug