Multiple Heteroatom-Hydrogen Bonds Bridging Electron Transport in Covalent Organic Framework-Based Supramolecular System for Photoreduction of CO2,Angewandte Chemie International Edition

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Multiple Heteroatom-Hydrogen Bonds Bridging Electron Transport in Covalent Organic Framework-Based Supramolecular System for Photoreduction of CO2
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-06-06 , DOI: 10.1002/anie.202307160
Yajun He ₁ , Yun Zhao ₁ , Xiaofeng Wang ₁ , Zheyuan Liu ₁ , Yan Yu ₁ , Liuyi Li ₁

Affiliation

A heteroatom-hydrogen bonds bridging electron transport pathway is revealed in a noncovalent-linked supramolecular photosystem, starting from readily available COF and metal-bipyridine complex. The hydrogen bonding supramolecular system exhibits enhanced electron transfer and performance for CO₂ photoreduction. This work provides an avenue to rationally design easily accessible photosystems.

中文翻译：

基于共价有机框架的超分子系统中桥接电子传输的多个杂原子-氢键用于 CO2 的光还原

在非共价连接的超分子光系统中揭示了桥接电子传输途径的杂原子-氢键，从容易获得的 COF 和金属-联吡啶络合物开始。氢键超分子系统表现出增强的电子转移和CO ₂光还原性能。这项工作为合理设计易于访问的光系统提供了一条途径。

更新日期：2023-06-06

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