Electrode/Electrolyte Synergy for Concerted Promotion of Electron and Proton Transfers toward Efficient Neutral Water Oxidation,Angewandte Chemie International Edition

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Electrode/Electrolyte Synergy for Concerted Promotion of Electron and Proton Transfers toward Efficient Neutral Water Oxidation
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-06-06 , DOI: 10.1002/anie.202303200
Yaming Hao ₁ , Yikun Kang ₁ , Shaoyan Wang ₁ , Zhe Chen ₁ , Can Lei ₁ , Xueting Cao ₁ , Lin Chen ₁ , Yefei Li ₁ , Zhipan Liu ₁ , Ming Gong ₁

Affiliation

An electrode/electrolyte synergy strategy is devised to enhance the neutral water oxidation. The concerted promotion of electron transfer via the IrO_x/NiOOH interface and proton transfer via the near-surface ion environment synergistically accelerated the proton-coupled electron transfer events. The expedited kinetics enabled the direct detection of oxygen intermediates at the electrode-electrolyte interface.

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