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Hydroxyl Radical-Mediated Efficient Photoelectrocatalytic NO Oxidation with Simultaneous Nitrate Storage Using A Flow Photoanode Reactor
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-05-16 , DOI: 10.1002/anie.202305538 Shuangjun Li 1 , Huan Shang 1, 2 , Ying Tao 1 , Pengpeng Li 2 , Honghui Pan 3 , Qing Wang 1 , Shao Zhang 1 , Hongbao Jia 2 , Haonan Zhang 1 , Jiazhen Cao 1 , Bixiang Zhang 1 , Rui Zhang 1 , Guisheng Li 2 , Yanrong Zhang 3 , Dieqing Zhang 1 , Hexing Li 1
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-05-16 , DOI: 10.1002/anie.202305538 Shuangjun Li 1 , Huan Shang 1, 2 , Ying Tao 1 , Pengpeng Li 2 , Honghui Pan 3 , Qing Wang 1 , Shao Zhang 1 , Hongbao Jia 2 , Haonan Zhang 1 , Jiazhen Cao 1 , Bixiang Zhang 1 , Rui Zhang 1 , Guisheng Li 2 , Yanrong Zhang 3 , Dieqing Zhang 1 , Hexing Li 1
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The Ni-modified NH2-UiO-66(Zr)/nickel foam with abundant mesoporous pores enables the progressive conversion of NO into nitrate without releasing remarkable NO2 by refining the reactive oxygen species to ⋅OH and can achieve the simultaneous storage of metabolic nitrogen for crop plants through a flow photoanode reactor. This study provides a state-of-the-art strategy for NO removal and sustainable nitrate storage.
中文翻译：
使用流动光阳极反应器进行羟基自由基介导的高效光电催化 NO 氧化并同时存储硝酸盐
具有丰富介孔的Ni改性NH 2 -UiO-66(Zr)/镍泡沫能够通过将活性氧精炼为·OH，将NO逐渐转化为硝酸盐，而不释放大量NO 2，并可以同时储存代谢物通过流动光电阳极反应器为农作物提供氮气。这项研究为去除 NO 和可持续硝酸盐储存提供了最先进的策略。
更新日期：2023-05-16
中文翻译：
使用流动光阳极反应器进行羟基自由基介导的高效光电催化 NO 氧化并同时存储硝酸盐
具有丰富介孔的Ni改性NH 2 -UiO-66(Zr)/镍泡沫能够通过将活性氧精炼为·OH，将NO逐渐转化为硝酸盐，而不释放大量NO 2，并可以同时储存代谢物通过流动光电阳极反应器为农作物提供氮气。这项研究为去除 NO 和可持续硝酸盐储存提供了最先进的策略。
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