Methane Carboxylation Using Electrochemically Activated Carbon Dioxide,Angewandte Chemie International Edition

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Methane Carboxylation Using Electrochemically Activated Carbon Dioxide
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-05-04 , DOI: 10.1002/anie.202305568
Yucheng Yuan ₁ , Yuhan Zhang ₁ , Haoyi Li ₁ , Muchun Fei ₁ , Hongna Zhang ₁ , John Santoro ₁ , Dunwei Wang ₁

Affiliation

Direct synthesis of CH₃COOH from CH₄ and CO₂ is made possible. The process first activates CO₂ by electrochemistry, producing CO and O₂. It is followed by oxidative CH₄ carbonylation catalyzed by Rh single atom catalysts. The net result is CH₄ carboxylation with 100 % atom economy.

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