Quantifying the Contribution of Hot Electrons in Photothermal Catalysis: A Case Study of Ammonia Synthesis over Carbon-supported Ru Catalyst,Angewandte Chemie International Edition

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Quantifying the Contribution of Hot Electrons in Photothermal Catalysis: A Case Study of Ammonia Synthesis over Carbon-supported Ru Catalyst
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-04-21 , DOI: 10.1002/anie.202304452
Xuanang Bian _{1,

2} , Yunxuan Zhao ₁ , Geoffrey I N Waterhouse ₃ , Yingxuan Miao _{1,

2} , Chao Zhou ₁ , Li-Zhu Wu ₁ , Tierui Zhang _{1,

2}

Affiliation

The actual reaction temperature of photothermal catalytic ammonia synthesis was determined according to Le Chatelier′s principle, enabling the contributions of hot-electron and local heating effects to be quantified separately. Further, we systematically investigated the hot-electron enhancement mechanism by disentangling the hot-electron effects from the local heating.

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