Overcoming Diffusion Limitation of Faradaic Processes: Property-Performance Relationships of 2D Conductive Metal-Organic Framework Cu3(HHTP)2 for Reversible Lithium-Ion Storage,Angewandte Chemie International Edition

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Overcoming Diffusion Limitation of Faradaic Processes: Property-Performance Relationships of 2D Conductive Metal-Organic Framework Cu3(HHTP)2 for Reversible Lithium-Ion Storage
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-04-17 , DOI: 10.1002/anie.202303111
Jens Matthies Wrogemann ₁ , Marco Joes Lüther ₁ , Peer Bärmann ₂ , Mailis Lounasvuori ₂ , Ali Javed ₃ , Michael Tiemann ₃ , Ronny Golnak ₂ , Jie Xiao ₂ , Tristan Petit ₂ , Tobias Placke ₁ , Martin Winter _{1,

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Affiliation

A two-dimensional MOF, (Cu₃(HHTP)₂), is synthesized with two different morphologies. Flake- and rod-like shaped particles were evaluated to investigate the impact of the particle morphology of MOFs on electrochemical Li⁺ ion storage. By optimization of the particle morphology, diffusion limitation of the Faradaic process can be strongly reduced.

中文翻译：

克服法拉第过程的扩散限制：用于可逆锂离子存储的二维导电金属有机骨架 Cu3(HHTP)2 的性能-性能关系

合成了具有两种不同形态的二维 MOF (Cu ₃ (HHTP) _{2 )。}评估了片状和棒状颗粒，以研究 MOF 的颗粒形态对电化学 Li ⁺离子存储的影响。通过优化粒子形态，可以大大降低法拉第过程的扩散限制。

更新日期：2023-04-17

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