Activating Lattice Oxygen in Spinel ZnCo2O4 through Filling Oxygen Vacancies with Fluorine for Electrocatalytic Oxygen Evolution,Angewandte Chemie International Edition

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Activating Lattice Oxygen in Spinel ZnCo2O4 through Filling Oxygen Vacancies with Fluorine for Electrocatalytic Oxygen Evolution
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-03-21 , DOI: 10.1002/anie.202301408
Kang Xiao ₁ , Yifan Wang ₂ , Peiyuan Wu ₁ , Liping Hou ₂ , Zhao-Qing Liu ₁

Affiliation

In this work, we successfully filled the lattice oxygen vacancies of ZnCo₂O₄ with F atom, achieving the activation of lattice oxygen by regulating metal-oxygen hybridization, and the dominant oxygen evolution reaction mechanism on ZnCo₂O₄ can transform from adsorbate evolution mechanism to lattice oxygen oxidation mechanism.

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