C-Bound or O-Bound Surface: Which One Boosts Electrocatalytic Urea Synthesis?,Angewandte Chemie International Edition

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C-Bound or O-Bound Surface: Which One Boosts Electrocatalytic Urea Synthesis?
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-03-09 , DOI: 10.1002/anie.202300387
Yingying Liu ₁ , Xiaojin Tu ₁ , Xiaoxiao Wei ₁ , Dongdong Wang ₁ , Xiaoran Zhang ₁ , Wei Chen ₁ , Chen Chen ₁ , Shuangyin Wang ₁

Affiliation

The electrocatalytic C−N coupling from carbon dioxide and nitrate is a sustainable and promising alternative for urea synthesis. Here we demonstrate that the localized negatively charged surface with C-affinity is superior to the positively charged one with O-affinity, providing guidance for screening and design of electrocatalysts for urea synthesis.

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