Regioisomeric Benzidine-Fullerenes: Tuning of the Diverse Hole-Distribution to Influence Charge Separation Patterns,Angewandte Chemie International Edition

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Regioisomeric Benzidine-Fullerenes: Tuning of the Diverse Hole-Distribution to Influence Charge Separation Patterns
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-02-15 , DOI: 10.1002/anie.202300377
Chong Wang _{1,

2} , Bo Wu _{1,

2} , Yang Li ₃ , Tianyang Dong _{1,

4} , Yongqiang Chai ₁ , Yuhe Zhang ₁ , Chunru Wang _{1,

2}

Affiliation

Three regioisomeric benzidine-fullerenes have been synthesized. Following charge separation (CS), the para-isomer manifests hole-delocalization, promoting ultrafast CS; while meta- and ortho-isomers cause hole-localization, contributing to long-lived CS state. This work reveals the influence of regioisomerism on charge distribution and CS.

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