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Organosulfur Materials for Rechargeable Batteries: Structure, Mechanism, and Application
Chemical Reviews ( IF 51.4 ) Pub Date : 2023-02-09 , DOI: 10.1021/acs.chemrev.2c00739 Pengfei Sang 1 , Qiliang Chen 1 , Dan-Yang Wang 1 , Wei Guo 1 , Yongzhu Fu 1
Chemical Reviews ( IF 51.4 ) Pub Date : 2023-02-09 , DOI: 10.1021/acs.chemrev.2c00739 Pengfei Sang 1 , Qiliang Chen 1 , Dan-Yang Wang 1 , Wei Guo 1 , Yongzhu Fu 1
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Lithium-ion batteries have received significant attention over the last decades due to the wide application of portable electronics and increasing deployment of electric vehicles. In order to further enhance the performance of the batteries and overcome the capacity limitations of inorganic electrode materials, it is imperative to explore new cathode and functional materials for rechargeable lithium batteries. Organosulfur materials containing sulfur–sulfur bonds as a kind of promising organic electrode materials have the advantages of high capacities, abundant resources, tunable structures, and environmental benignity. In addition, organosulfur materials have been widely used in almost every aspect of rechargeable batteries because of their multiple functionalities. This review aims to provide a comprehensive overview on the development of organosulfur materials including the synthesis and application as cathode materials, electrolyte additives, electrolytes, binders, active materials in lithium redox flow batteries, and other metal battery systems. We also give an in-depth analysis of structure–property–performance relationship of organosulfur materials, and guidance for the future development of organosulfur materials for next generation rechargeable lithium batteries and beyond.
中文翻译：
可充电电池用有机硫材料：结构、机理和应用
在过去的几十年里，由于便携式电子产品的广泛应用和电动汽车的日益普及，锂离子电池受到了极大的关注。为了进一步提升电池的性能并克服无机电极材料的容量限制，探索新型可充电锂电池正极和功能材料势在必行。含有硫-硫键的有机硫材料作为一种有前景的有机电极材料，具有容量高、资源丰富、结构可调、环境友好等优点。此外，有机硫材料因其多功能性而被广泛应用于可充电电池的几乎各个方面。本综述旨在全面概述有机硫材料的发展，包括作为正极材料、电解液添加剂、电解质、粘合剂、锂氧化还原液流电池和其他金属电池系统中的活性材料的合成和应用。我们还深入分析了有机硫材料的结构-性能-性能关系，为下一代可充电锂电池及其他有机硫材料的未来发展提供指导。
更新日期：2023-02-09
中文翻译：
可充电电池用有机硫材料：结构、机理和应用
在过去的几十年里，由于便携式电子产品的广泛应用和电动汽车的日益普及，锂离子电池受到了极大的关注。为了进一步提升电池的性能并克服无机电极材料的容量限制，探索新型可充电锂电池正极和功能材料势在必行。含有硫-硫键的有机硫材料作为一种有前景的有机电极材料，具有容量高、资源丰富、结构可调、环境友好等优点。此外，有机硫材料因其多功能性而被广泛应用于可充电电池的几乎各个方面。本综述旨在全面概述有机硫材料的发展，包括作为正极材料、电解液添加剂、电解质、粘合剂、锂氧化还原液流电池和其他金属电池系统中的活性材料的合成和应用。我们还深入分析了有机硫材料的结构-性能-性能关系，为下一代可充电锂电池及其他有机硫材料的未来发展提供指导。
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