A Triptycene-Based 2D MOF with Vertically Extended Structure for Improving the Electrocatalytic Performance of CO2 to Methane,Angewandte Chemie International Edition

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A Triptycene-Based 2D MOF with Vertically Extended Structure for Improving the Electrocatalytic Performance of CO2 to Methane
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-01-24 , DOI: 10.1002/anie.202217958
Jianning Lv ₁ , Wenrui Li ₁ , Jiani Li ₁ , Zhejiaji Zhu ₁ , Anwang Dong ₁ , Huixia Lv ₁ , Pengfei Li ₁ , Bo Wang _{1,

2}

Affiliation

A two-dimensional vertically conductive metal-organic framework (2D-vc-MOF(Cu)) was designed and synthesized with a hexahydroxyltriptycene ligand, which features a vertically extended structure. The 2D-vc-MOF(Cu) exhibits a two-fold Faradaic efficiency improvement compared to the planarly extended 2D conductive MOFs, displaying the potential of the structural design in the catalytic performance enhancement.

中文翻译：

具有垂直延伸结构的基于三蝶烯的二维 MOF 用于提高 CO2 制甲烷的电催化性能

设计并合成了具有垂直延伸结构的六羟基三蝶烯配体的二维垂直导电金属有机骨架 (2D- vc -MOF(Cu))。与平面延伸的 2D 导电 MOF 相比， 2D- vc -MOF(Cu) 的法拉第效率提高了两倍，显示出结构设计在提高催化性能方面的潜力。

更新日期：2023-01-24

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