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Organic Additive-derived Films on Cu Electrodes Promote Electrochemical CO2 Reduction to C2+ Products Under Strongly Acidic Conditions
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2023-01-19 , DOI: 10.1002/anie.202216102
Weixuan Nie 1 , Gavin P Heim 1 , Nicholas B Watkins 1 , Theodor Agapie 1 , Jonas C Peters 1
Affiliation  

Modified copper electrodes with N-tolyl pyridinium additive-derived films show boosted selectivity of the CO2 reduction to C2+ products (>70 % Faradaic efficiency) and great suppression of the hydrogen evolution reaction in strongly acidic electrolytes with low alkali cation concentrations.

中文翻译:

Cu 电极上的有机添加剂衍生膜在强酸性条件下促进电化学 CO2 还原为 C2+ 产物

具有 N-甲苯基吡啶添加剂衍生薄膜的改性铜电极显示出将 CO 2还原为 C 2+产物的选择性提高(>70% 法拉第效率),并且在具有低碱阳离子浓度的强酸性电解质中显着抑制析氢反应。
更新日期:2023-01-19
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