Leveraging Crystalline and Amorphous States of a Metal-Organic Complex for Transformation of the Photosalient Effect and Positive-Negative Photochromism,Angewandte Chemie International Edition

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Leveraging Crystalline and Amorphous States of a Metal-Organic Complex for Transformation of the Photosalient Effect and Positive-Negative Photochromism
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-12-26 , DOI: 10.1002/anie.202217054
Yu-Juan Ma ₁ , Guowei Xiao ₁ , Xiaoyu Fang ₁ , Tianhong Chen ₁ , Dongpeng Yan ₁

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An approach to leverage crystalline and amorphous states of a zero-dimensional metal-organic complex in order to tune negative and positive photochromism was proposed, which could be assigned to the competitive chemical routes between photocycloaddition and photogenerated radicals. Furthermore, both polymorphs exhibit mechanochromic photoemission, and lead to the on/off toggling of the light-driven motion of bulky molecular crystals.

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