In Situ Formation of Nitrogen-Rich Solid Electrolyte Interphase and Simultaneous Regulating Solvation Structures for Advanced Zn Metal Batteries,Angewandte Chemie International Edition

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In Situ Formation of Nitrogen-Rich Solid Electrolyte Interphase and Simultaneous Regulating Solvation Structures for Advanced Zn Metal Batteries
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-11-02 , DOI: 10.1002/anie.202212839
Dongdong Wang ₁ , Dan Lv ₁ , Hongxia Liu ₂ , Shaojie Zhang ₁ , Cheng Wang ₁ , Chunting Wang ₁ , Jian Yang ₁ , Yitai Qian _{1,

3}

Affiliation

A bifunctional electrolyte additive, N-Methyl pyrrolidone (NMP), is developed to improve the electrochemical performance of Zn anodes. NMP not only alters the solvation structure of Zn²⁺, but also in situ produces a dense nitrogen-rich layer on Zn. This layer protects Zn from corrosive electrolytes and benefits the uniform plating/stripping of Zn.

中文翻译：

富氮固体电解质中间相的原位形成和先进锌金属电池的同步调节溶剂化结构

开发了一种双功能电解质添加剂 N-甲基吡咯烷酮 (NMP)，以提高锌阳极的电化学性能。NMP不仅改变了Zn ²⁺的溶剂化结构，而且在Zn上原位产生致密的富氮层。该层保护 Zn 免受腐蚀性电解质的影响，并有利于 Zn 的均匀电镀/剥离。

更新日期：2022-11-02

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