Side-Chain Control of Topochemical Polymer Single Crystals with Tunable Elastic Modulus,Angewandte Chemie International Edition

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Side-Chain Control of Topochemical Polymer Single Crystals with Tunable Elastic Modulus
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-10-11 , DOI: 10.1002/anie.202213840
Zitang Wei ₁ , Xiaokang Wang ₂ , Bumjoon Seo ₁ , Xuyi Luo ₁ , Qixuan Hu ₁ , Jack Jones ₁ , Matthias Zeller ₃ , Kang Wang ₁ , Brett M Savoie ₁ , Kejie Zhao ₂ , Letian Dou _{1,

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Affiliation

Topochemically reactive single crystals of bis(indandione) derivatives were carefully functionalized by controlling side chain length as well as introducing different end groups on the side chains. While maintaining topochemical reactivities, modifying side chains can significantly affect polymerization kinetics and enhance polymer elastic modulus. Furthermore, polymer single crystals could be processed into free-standing and robust thin films.

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