The Progress and Outlook of Metal Single-Atom-Site Catalysis,Journal of the American Chemical Society

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The Progress and Outlook of Metal Single-Atom-Site Catalysis
Journal of the American Chemical Society ( IF 14.4 ) Pub Date : 2022-09-29 , DOI: 10.1021/jacs.1c12642
Xiao Liang ₁ , Ninghua Fu ₁ , Shuangchao Yao ₁ , Zhi Li _{1,

2} , Yadong Li _{1,

2,

3}

Affiliation

Single-atom-site catalysts (SASCs) featuring maximized atom utilization and isolated active sites have progressed tremendously in recent years as a highly prosperous branch of catalysis research. Varieties of SASCs have been developed that show excellent performance in many catalytic applications. The major goal of SASC research is to establish feasible synthetic strategies for the preparation of high-performance catalysts, to achieve an in-depth understanding of the active-site structures and catalytic mechanisms, and to develop practical catalysts with industrial value. This Perspective describes the up-to-date development of SASCs and related catalysts, such as dual-atom-site catalysts (DASCs) and nano-single-atom-site catalysts (NSASCs), analyzes the current challenges encountered by these catalysts for industrial applications, and proposes their possible future development path.

中文翻译：

金属单原子位催化的进展与展望

近年来，具有最大化原子利用率和孤立活性位点的单原子位点催化剂（SASCs）作为催化研究的一个非常繁荣的分支取得了长足的进步。已开发出多种 SASC，它们在许多催化应用中表现出优异的性能。SASC研究的主要目标是为制备高性能催化剂建立可行的合成策略，深入了解活性位点结构和催化机理，开发具有工业价值的实用催化剂。本文介绍了双原子位点催化剂 (DASCs) 和纳米单原子位点催化剂 (NSASCs) 等 SASCs 和相关催化剂的最新发展，分析了这些催化剂在工业领域所面临的当前挑战应用，

更新日期：2022-09-29

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