Enhancing Hydrogen Oxidation and Evolution Kinetics by Tuning the Interfacial Hydrogen-Bonding Environment on Functionalized Platinum Surfaces,Angewandte Chemie International Edition

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Enhancing Hydrogen Oxidation and Evolution Kinetics by Tuning the Interfacial Hydrogen-Bonding Environment on Functionalized Platinum Surfaces
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-08-08 , DOI: 10.1002/anie.202207197
Kaiyue Zhao ₁ , Xiaoxia Chang ₁ , Hai-Sheng Su ₁ , Yiming Nie ₂ , Qi Lu ₃ , Bingjun Xu ₁

Affiliation

Specifically adsorbed organic additives are found to enhance the intrinsic kinetics of hydrogen evolution and oxidation reactions in alkaline solution on Pt surfaces by reorganizing the interfacial water structure. In situ vibrational spectroscopies present compelling evidence that weakly hydrogen-bonded water has a substantial impact on the hydrogen electrocatalytic process.

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