Bioinspired Photocatalytic NADH Regeneration by Covalently Metalated Carbon Nitride for Enhanced CO2 Reduction,Chemistry - A European Journal

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Bioinspired Photocatalytic NADH Regeneration by Covalently Metalated Carbon Nitride for Enhanced CO2 Reduction
Chemistry - A European Journal ( IF 3.9 ) Pub Date : 2022-06-27 , DOI: 10.1002/chem.202201430
Yuanyuan Zhang _{1,

2} , Jian Liu _{1,

2}

Affiliation

An artificial photosystem was constructed through the covalent attachment of Rh complex onto PCN. The integrated photocatalyst could regenerate NADH efficiently by integrating the light harvesting unit and the electron transfer unit through conjugated connection. By further coupling with FDH immobilized on the hydrophobic membrane, an enhanced HCOOH production could be obtained.

中文翻译：

Bioinspired 共价金属化碳氮化物光催化 NADH 再生增强 CO2 还原

通过将 Rh 复合物共价连接到 PCN 上，构建了一个人工光系统。集成光催化剂可以通过共轭连接将光收集单元和电子转移单元集成在一起，从而有效地再生NADH。通过进一步与固定在疏水膜上的 FDH 偶联，可以获得增强的 HCOOH 产量。

更新日期：2022-06-27

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