Steering Catalytic Activity and Selectivity of CO2 Photoreduction to Syngas with Hydroxy-Rich Cu2S@ROH-NiCo2O3 Double-Shelled Nanoboxes,Angewandte Chemie International Edition

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Steering Catalytic Activity and Selectivity of CO2 Photoreduction to Syngas with Hydroxy-Rich Cu2S@ROH-NiCo2O3 Double-Shelled Nanoboxes
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-06-13 , DOI: 10.1002/anie.202205839
Lei Li ₁ , Xinyan Dai ₂ , De-Li Chen ₁ , Yinxiang Zeng ₃ , Yong Hu _{1,

2} , Xiong Wen David Lou ₃

Affiliation

Hierarchical Cu₂S@R_OH-NiCo₂O₃ double-shelled nanoboxes are synthesized through a multistep strategy to regulate the activity and selectivity of CO₂ photoreduction into syngas. The hierarchical hollow structure and p–n heterojunction enable enhanced light absorption and fast charge separation. Moreover, the catalytic activity can be tuned by controlling the content of hydroxy groups on the surfaces of R_OH-NiCo₂O₃.

中文翻译：

用富羟基 Cu2S@ROH-NiCo2O3 双壳纳米盒指导 CO2 光还原制合成气的催化活性和选择性

通过多步策略合成分级Cu ₂ S@ R _OH -NiCo ₂ O ₃双壳纳米盒，以调节CO ₂光还原为合成气的活性和选择性。分层中空结构和 p-n 异质结能够增强光吸收和快速电荷分离。此外，可以通过控制R _OH -NiCo ₂ O ₃表面的羟基含量来调节催化活性。

更新日期：2022-06-13

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