Lattice-Confined Single-Atom Fe1Sx on Mesoporous TiO2 for Boosting Ambient Electrocatalytic N2 Reduction Reaction,Angewandte Chemie International Edition

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Lattice-Confined Single-Atom Fe1Sx on Mesoporous TiO2 for Boosting Ambient Electrocatalytic N2 Reduction Reaction
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-04-12 , DOI: 10.1002/anie.202203022
Jiayin Chen ₁ , Yikun Kang ₁ , Wei Zhang _{1,

2} , Zhenghao Zhang ₁ , Yan Chen ₁ , Yi Yang ₁ , Linlin Duan ₁ , Yefei Li ₁ , Wei Li ₁

Affiliation

S-coordinated Fe single-atom catalysts on mesoporous TiO₂ have been constructed by a universal lattice-confined strategy. This catalyst shows a unique nanoconfinement effect for the mass transfer and maximizes the active sites to mimic nitrogenase for ambient electrocatalytic N₂ reduction reaction.

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