Recent Progress of Metal Organic Frameworks-Based Electrocatalysts for Hydrogen Evolution, Oxygen Evolution, and Oxygen Reduction Reaction,Energy & Environmental Materials

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Recent Progress of Metal Organic Frameworks-Based Electrocatalysts for Hydrogen Evolution, Oxygen Evolution, and Oxygen Reduction Reaction
Energy & Environmental Materials ( IF 13.0 ) Pub Date : 2021-10-15 , DOI: 10.1002/eem2.12290
Yaling Jia ₁ , Ziqian Xue ₂ , Yinle Li ₁ , Guangqin Li ₁ , Z. Xue ₂

Affiliation

Exploring efficient and cost-saving electrocatalysts is essential to the renewable energy storage and utilization, which is still in its embryonic period. MOFs have drawn tremendous attention due to their adjustability, abundant active sites, and plentiful pores. Notably, satisfactory electrocatalytic performance has been achieved by MOFs-based electrocatalysts comparable to traditional electrocatalysts. State-of-the-art works about the MOFs-based electrocatalysts for hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and ORR were summarized in this review. This review comprises a series of modifying strategies of MOFs and their derivatives, from aspects of structure, composition, and morphology. Furthermore, the active sites and functional mechanisms’ recognition are involved in this review expecting to provide reference for rationally designing efficient electrocatalysts. At last, the current status, challenges, and perspectives of MOFs-based electrocatalysts are also discussed.

中文翻译：

基于金属有机骨架的析氢、析氧和氧还原反应电催化剂的最新进展

探索高效、节约成本的电催化剂对于可再生能源的存储和利用至关重要，而可再生能源仍处于萌芽期。MOFs由于其可调节性、丰富的活性位点和丰富的孔隙而引起了极大的关注。值得注意的是，与传统电催化剂相当的基于 MOF 的电催化剂已经实现了令人满意的电催化性能。本综述总结了基于 MOFs 的用于析氢反应 (HER)、析氧反应 (OER) 和 ORR 的电催化剂的最新进展。本综述包括从结构、组成和形态等方面对 MOF 及其衍生物的一系列修饰策略。此外，本综述涉及活性位点和功能机制的识别，希望为合理设计高效电催化剂提供参考。最后，还讨论了基于 MOFs 的电催化剂的现状、挑战和前景。

更新日期：2021-10-15

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