Engineering Olefin-Linked Covalent Organic Frameworks for Photoenzymatic Reduction of CO2,Angewandte Chemie International Edition

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Engineering Olefin-Linked Covalent Organic Frameworks for Photoenzymatic Reduction of CO2
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-01-18 , DOI: 10.1002/anie.202200261
Zhengfeng Zhao _{1,

2,

3} , Dong Zheng _{1,

2} , Menglei Guo _{1,

2} , Jiangyue Yu _{1,

2} , Sainan Zhang _{1,

2} , Zhenjie Zhang _{1,

4} , Yao Chen _{1,

2}

Affiliation

A new photocatalyst–enzyme coupled artificial photosynthesis system was constructed for photoenzymatic reduction of CO₂ using COFs as enzyme carriers. The hybrid system showed an apparent quantum yield as high as 9.17±0.44 %, surpassing the reported NADH-regenerated photocatalysts of crystalline framework materials.

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